PhD defense
Attosecond science has revolutionized the ability to capture extremely fast phenomena in nature, opening a window into a new temporal regime, in which electron dynamics are observed on their natural time scale (1 as = 10-18 sec). Attosecond metrology relies on the ability to produce optical pulses, having attosecond duration, imprinting the electronic dynamics in their spectral intensity, phase and polarization state. However, the optical measurement resolves only the spectral intensity while the phase and polarization information are lost, preventing a direct access to the full information encoded in the attosecond signal.
In this talk, I will describe the application of one of the most fundamental optical schemes, interferometry, in the attosecond timescale [1,2]. Extending this scheme to the dynamic regime has unlocked new and exciting horizons in attosecond science. Time-resolved attosecond interferometry probes the evolution of an electronic wavefunction under the tunneling barrier, as it propagates in a classically forbidden region [3]. Its application to light-driven quantum systems decouples and follows the temporal evolution of individual underlying quantum paths with unprecedented precision and reveals the sub-cycle vectorial properties of transient light-matter interactions [4,5].
1. Azoury, D., Kneller, O., et al. Electronic wavefunctions probed by all-optical attosecond interferometry. Nature Photon 13, 54–59 (2019).
2. Azoury*, D., Kneller*, O. et al. Interferometric attosecond lock-in measurement of extreme-ultraviolet circular dichroism. Nature Photon 13, 198–204 (2019).
3. Kneller, O. et al. A look under the tunnelling barrier via attosecond-gated interferometry. Nat. Photon. 16, 304–310 (2022).
4. Kneller*, O., Mor*, C., Klimkin*, N.D. et al. Attosecond transient interferometry. Nat. Photon. 19, 134–141 (2025).
5. Kneller, O. et al. Attosecond Fourier transform spectroscopy. Submitted (2025).