Publications

Coherent optical memories will likely play an important role in future quantum communication networks. Among the different platforms, memories based on ladder-type orbital transitions in atomic gasses offer high bandwidth (>100 MHz), continuous (on-demand) readout, and low-noise operation. Here we report on an upgraded setup of our previously-reported fast ladder memory, with improved efficiency and lifetime, and reduced noise. The upgrade employs a stronger control field, wider signal beam, reduced atomic density, higher optical depth, annular optical-pumping beam, and weak dressing of an auxiliary orbital to counteract residual Doppler-broadening. For a 2 ns-long pulse, we demonstrate 53% internal efficiency, 35% end-to-end efficiency, 3 × 10⁻⁵ noise photons per pulse, and a 1/e lifetime of 108 ns. This combination of performances is a record for continuous-readout memories.

Vortices are topologically nontrivial defects that generally originate from nonlinear field dynamics. All-optical generation of photonic vortices-phase singularities of the electromagnetic field-requires sufficiently strong nonlinearity that is typically achieved in the classical optics regime. We report on the realization of quantum vortices of photons that result from a strong photon-photon interaction in a quantum nonlinear optical medium. The interaction causes faster phase accumulation for copropagating photons, producing a quantum vortex-antivortex pair within the two-photon wave function. For three photons, the formation of vortex lines and a central vortex ring confirms the existence of a genuine three-photon interaction. The wave function topology, governed by two- and three-photon bound states, imposes a conditional phase shift of π per photon, a potential resource for deterministic quantum logic operations.

We present general guidelines for finding solid-state systems that could serve as coherent electron-spin-photon interfaces even at relatively high temperatures, where phonons are abundant but cooling is easier, and show that transition-metal ions in various crystals could comply with these guidelines. As an illustrative example, we focus on divalent nickel ions in magnesium oxide. We perform electron-spin-resonance spectroscopy and polarization-sensitive magneto-optical fluorescence spectroscopy of a dense ensemble of these ions and find that (i) the ground-state electron spin stays coherent at liquid-helium temperatures for several microseconds and (ii) there exist energetically well-isolated excited states that can couple to two ground-state spin sublevels via optical transitions of orthogonal polarizations. The latter implies that fast coherent optical control over the electron spin is possible. We then propose schemes for optical initialization and control of the ground-state electron spin using polarized optical pulses, as well as two schemes for implementing a noise-free broadband quantum optical memory at near-telecom wavelengths in this material system.

We propose heat machines that are nonlinear, coherent, and closed systems composed of few field (oscillator) modes. Their thermal-state input is transformed by nonlinear Kerr interactions into nonthermal (non-Gaussian) output with controlled quantum fluctuations and the capacity to deliver work in a chosen mode. These machines can provide an output with strongly reduced phase and amplitude uncertainty that may be useful for sensing or communications in the quantum domain. They are experimentally realizable in optomechanical cavities where photonic and phononic modes are coupled by a Josephson qubit or in cold gases where interactions between photons are transformed into dipole-dipole interacting Rydberg atom polaritons. This proposed approach is a step toward the bridging of quantum and classical coherent and thermodynamic descriptions.

In recent works, we have put forth and experimentally demonstrated several novel schemes [1-5] for the detection of quantum noise signatures by exploiting frequent photonic measurements, allowing us to reach unprecedented, ultrahigh sensitivity to quantum noise.

Nuclear spins of noble gases can maintain coherence for hours at ambient conditions because they are isolated by complete electron shells¹. This isolation, however, impedes the ability to manipulate and control them by optical means or by coupling to other spin gases²⁴. Here we achieve strong coherent coupling between noble-gas spins and the optically accessible spins of an alkali-metal vapour. The coupling emerges from the coherent accumulation of stochastic spin-exchange collisions. We obtain a coupling strength ten times higher than the decay rate, observe the coherent and periodic exchange of spin excitations between the two gases and demonstrate active control over the coupling by an external magnetic field. This approach could be developed into a fast and efficient interface for noble-gas spins, enabling applications in quantum sensing and information^5,6.

An ensemble of noble-gas nuclear spins is a unique quantum system that could maintain coherence for many hours at room temperature and above, owing to exceptional isolation from the environment. This isolation, however, is a mixed blessing, limiting the ability of these ensembles to interface with other quantum systems coherently. Here we show that spin-exchange collisions with alkali-metal atoms render a quantum interface for noble-gas spins without impeding their long coherence times. We formulate the many-body theory of the hybrid system and reveal a collective mechanism that strongly couples the macroscopic quantum states of the two spin ensembles. Despite their stochastic and random nature, weak collisions enable entanglement and reversible exchange of nonclassical excitations in an efficient, controllable, and deterministic process. With recent experiments now entering the strong-coupling regime, this interface paves the way toward realizing hour-long quantum memories and entanglement at room temperature.

We propose a novel principle of operating heat machines in a fully unitary (coherent) fashion by mixing few hot and cold thermal field modes in nonlinear interferometers. Such devices, specifically, interferometers containing Kerr-nonlinear intermode cross-couplers, are shown to enable autonomous concentration of the energy predominantly in a desired output mode, at the expense of the other modes. Their phase-coherent operation is reversible and it is approximately reversible even if intermode entanglement is neglected. Such few-mode coherent heat machines radically depart from the existing thermodynamic paradigm which treats heat machines as open systems dissipated by heat baths.

Photonic measurement-based quantum computation (MBQC) is a promising route towards fault-tolerant universal quantum computing. A central challenge in this effort is the huge overhead in the resources required for the construction of large photonic clusters using probabilistic linear-optics gates. Although strong single-photon nonlinearity ideally enables deterministic construction of such clusters, it is challenging to realise in a scalable way. Here we explore the prospects of using moderate nonlinearity (with conditional phase shifts smaller than π ) to boost photonic quantum computing and significantly reduce its resources overhead. The key element in our scheme is a nonlinear router that preferentially directs photonic wavepackets to different output ports depending on their intensity. As a relevant example, we analyze the nonlinearity provided by Rydberg blockade in atomic ensembles, in which the trade-off between the nonlinearity and the accompanying loss is well understood. We present protocols for efficient Bell measurement and GHZ-state preparationboth key elements in the construction of cluster states, as well as for the cnot gate and quantum factorization. Given the large number of entangling operations involved in fault-tolerant MBQC, the increase in success probability provided by our protocols already at moderate nonlinearities can result in a significant reduction in the required resources.

Nuclear spins of noble gases feature extremely long coherence times but are inaccessible to optical photons. Here, we realize a coherent interface between light and noble-gas spins that is mediated by alkali atoms. We demonstrate the optical excitation of the noble-gas spins and observe the coherent back action on the light in the form of high-contrast two-photon spectra. We report on a record two-photon linewidth of 5 ± 0.7 mHz above room temperature, corresponding to a 1-min coherence time. This experiment provides a demonstration of coherent bidirectional coupling between light and noble-gas spins, rendering their long-lived spin coherence accessible for manipulations in the optical domain.

We introduce and demonstrate a scheme for eliminating the inhomogeneous dephasing of a collective quantum state. The scheme employs off-resonant fields that continuously dress the collective state with an auxiliary sensor state, which has an enhanced and opposite sensitivity to the same source of inhomogeneity. We derive the optimal conditions under which the dressed state is fully protected from dephasing when using either one or two dressing fields. The latter provides better protection, circumvents qubit phase rotation, and suppresses the sensitivity to drive noise. We further derive expressions for all residual, higher-order sensitivities. We experimentally study the scheme by protecting a collective excitation of an atomic ensemble, where inhomogeneous dephasing originates from thermal motion. Using photon storage and retrieval, we demonstrate complete suppression of inhomogeneous dephasing and, consequently, a prolonged memory time. Our scheme may be applied to eliminate motional dephasing in other systems, improving the performance of quantum gates and memorieswith neutral atoms. It is also generally applicable to various gas, solid, and engineered systems, where sensitivity to variations in time, space, or other domains limits possible scale-up of the system.

Bessel beams are renowned members of a wide family of non-diffracting (propagationinvariant) fields. We report on experiments showing that non-diffracting fields are also immune to diffusion. We map the phase and magnitude of structured laser fields onto the spatial coherence between two internal states of warm atoms undergoing diffusion. We measure the field after a controllable, effective, diffusion time by continuously generating light from the spatial coherence. The coherent diffusion of Bessel-Gaussian fields and more intricate, non-diffracting fields is quantitatively analyzed and directly compared to that of diffracting fields. To elucidate the origin of diffusion invariance, we show results for non-diffracting fields whose phase pattern we flatten.

Optical quantum memories, which store and preserve the quantum state of photons, rely on a coherent mapping of the photonic state onto matter states that are optically accessible. Here we outline a new physical mechanism to map the state of photons onto the long-lived but optically inaccessible collective state of noble-gas spins. The mapping employs the coherent spin-exchange interaction arising from random collisions with alkali vapor. We analyze optimal strategies for high-efficiency storage and retrieval of non-classical light at various parameter regimes. Based on these strategies, we identify feasible experimental conditions for realizing efficient quantum memories with noble-gas spins having hours-long coherence times at room temperature and above

The Fresnel-Fizeau effect of transverse drag, in which the trajectory of a light beam changes due to transverse motion of the optical medium, is usually extremely small and hard to detect. We observe transverse drag in a moving hot-vapor cell, utilizing slow light due to electromagnetically induced transparency (EIT). The drag effect is enhanced by a factor 400,000, corresponding to the ratio between the light speed in vacuum and the group velocity under the EIT conditions. We study the contribution of the thermal atomic motion, which is much faster than the mean medium velocity, and identify the regime where its effect on the transverse drag is negligible.

Point-source atom interferometry is a promising approach for implementing robust, high-sensitivity, rotation sensors using cold atoms. However, its scale factor, i.e., the ratio between the interferometer signal and the actual rotation rate, depends on the initial conditions of the atomic cloud, which may drift in time and result in bias instability, particularly in compact devices with short interrogation times. We present two methods to stabilize the scale factor. One relies on a model-based correction which exploits correlations between multiple features of the interferometer output and works on a single-shot basis. The other is a self-calibrating method where a known bias rotation is applied to every other measurement, requiring no prior knowledge of the underlying model but reducing the sensor bandwidth by a factor of two. We demonstrate both schemes experimentally with complete suppression of scale-factor drifts, maintaining the original rotation sensitivity and allowing for bias-free operation over several hours.

We introduce and demonstrate a scheme for eliminating the inhomogeneous dephasing of a collective quantum state. The scheme employs off-resonant optical fields that dress the collective state with an auxiliary sensor state, which has an enhanced and opposite sensitivity to the same source of inhomogeneity. We derive the optimal conditions under which the dressed state is fully protected from dephasing, when using either one or two dressing fields. The latter provides better protection, prevents global phase rotation, and suppresses the sensitivity to drive noise. We further provide expressions for all residual, higher-order, sensitivities. We experimentally study the scheme by protecting a collective excitation of an atomic ensemble, where inhomogeneous dephasing originates from thermal motion. Using photon storage and retrieval, we demonstrate complete suppression of inhomogeneous dephasing and consequently a prolonged memory time. Our scheme may be applied to eliminate motional dephasing in other systems, improving the performance of quantum gates and memories with neutral atoms. It is also generally applicable to various gas, solid, and engineered systems, where sensitivity to variations in time, space, or other domains limits possible scale-up of the system.

Doppler broadening in thermal ensembles degrades the absorption cross-section and the coherence time of collective excitations. In two photon transitions, it is common to assume that this problem becomes worse with larger wavelength mismatch. Here we identify an opposite mechanism, where such wavelength mismatch leads to cancellation of Doppler broadening via the counteracting effects of velocity-dependent light-shifts and Doppler shifts. We show that this effect is general, common to both absorption and transparency resonances, and favorably scales with wavelength mismatch. We experimentally confirm the enhancement of transitions for different low-lying orbitals in rubidium atoms and use calculations to extrapolate to high-lying Rydberg orbitals. These calculations predict a dramatic enhancement of up to 20-fold increase in absorption, even in the presence of large homogeneous broadening. More general configurations, where an auxiliary dressing field is used to counteract Doppler broadening, are also discussed and experimentally demonstrated. The mechanism we study can be applied as well for rephasing of spin waves and increasing the coherence time of quantum memories.

Partially coherent fields are abundant in many physical systems. While the propagation of partially coherent light undergoing diffraction is well understood, its evolution in the presence of coherent diffusion (i.e., diffusion of complex fields) remains largely unknown. Here we develop an analytic model describing the diffusion of partially coherent beams and study it experimentally. Our model is based on a diffusion analog of the famous Van CittertZernike theorem. Experimentally, we use a four-wave mixing scheme with electromagnetically induced transparency to couple optical speckle patterns to diffusing atoms in a warm vapor. The spatial coherence properties of the speckle fields are monitored under diffusion and are compared to our model and to the familiar evolution of spatial coherence of light speckles under diffraction. We identify several important differences between the evolution dynamics of the spatial coherence under diffraction and diffusion. Our findings shed light on the propagation of partially coherent fields in media where multiple scattering or thermal motion lead to coherent diffusion.

Optical pumping is an efficient method for initializing and maintaining atomic spin ensembles in a well-defined quantum spin state. Standard optical pumping methods orient the spins by transferring photonic angular momentum to spin polarization. Generally the spins are oriented along the propagation direction of the light due to selection rules of the dipole interaction. Here we present and experimentally demonstrate that by modulating the light polarization, angular momentum perpendicular to the optical axis can be transferred efficiently to cesium vapor. The transverse pumping scheme employs transversely oriented dark states, allowing for control of the trajectory of the spins on the Bloch sphere. This new mechanism is suitable and potentially beneficial for diverse applications, particularly in quantum metrology.

Future quantum photonic networks require coherent optical memories for synchronizing quantum sources and gates of probabilistic nature. Room temperature operation is also desirable for ease of scaling up. Until now, however, room-temperature atomic memories have suffered from an intrinsic read-out noise due to spontaneous four-wave-mixing. Here we demonstrate a new scheme for storing photons at room temperature, the fast ladder memory (FLAME). In this scheme, stimulated two-photon absorption is used instead of the previously used stimulated Raman scattering. As here the competing spontaneous processes would require spontaneous absorption of an optical photon, rather than emission, the noise is greatly suppressed. Furthermore, high external efficiency can be achieved as the control is well separated in frequency from the signal, and could be filtered out using highly efficient interference filters. We run the protocol in rubidium vapour, both on and off single-photon resonance, demonstrating a ratio of 50 between storage time and signal pulse width, an external total efficiency of over 25%, and only 2.3 × 10 ^-4 noise photons per extracted signal photon. This paves the way towards the efficient synchronization of probabilistic gates and sources at room temperature, and the controlled production of large quantum states of light.

The spins of gaseous alkali-metal atoms are commonly assumed to oscillate at a constant hyperfine frequency, which for many years has been used to define a standard unit of time, the second. Indeed, under standard experimental conditions, the spins oscillate independently, only weakly perturbed and slowly decaying due to random spin-spin collisions. Here we consider a different, unexplored regime of very dense gas, where collisions, more frequent than the hyperfine frequency, dominate the dynamics. We find that the hyperfine oscillations become significantly longer lived, and their frequency becomes dependent on the state of the ensemble, manifesting strong nonlinear dynamics. We reveal that the nonlinearity originates from a many-body interaction which synchronizes the electronic spins, driving them into a single collective mode. The conditions for experimental realizations of this regime are outlined.

Future quantum photonic networks require coherent opticalmemories for synchronizing quantum sources and gates of probabilistic nature. We demonstrate a fast ladder memory (FLAME) mapping the optical field onto the superposition between electronic orbitals of rubidium vapor. Using a ladder-level system of orbital transitions with nearly degenerate frequencies simultaneously enables high bandwidth, low noise, and long memory lifetime. We store and retrieve 1.7-ns-long pulses, containing 0.5 photons on average, and observe short-time external efficiency of 25%, memory lifetime (1/e) of 86 ns, and below 10(-4) added noise photons. Consequently, coupling this memory to a probabilistic source would enhance the on-demand photon generation probability by a factor of 12, the highest number yet reported for a noise-free, room temperature memory. This paves the way toward the controlled production of large quantum states of light from probabilistic photon sources.

We use a four-wave mixing process to read-out light from atomic coherence which is continuously written. The light is continuously generated after an effective delay, allowing the atomic coherence to evolve during the process. Contrary to slow-light delay, which depends on the medium optical depth, here the generation delay is determined solely by the intensive properties of the system, approaching the atomic coherence lifetime at the weak driving limit. The atomic evolution during the generation delay is further manifested in the spatial profile of the generated light due to atomic diffusion. Continuous generation of light with a long intrinsic delay can replace discrete write-read procedures when the atomic evolution is the subject of interest.

The strong interaction between individual Rydberg atoms provides a powerful tool exploited in an ever-growing range of applications in quantum information science, quantum simulation and ultracold chemistry. One hallmark of the Rydberg interaction is that both its strength and angular dependence can be fine-tuned with great flexibility by choosing appropriate Rydberg states and applying external electric and magnetic fields. More and more experiments are probing this interaction at short atomic distances or with such high precision that perturbative calculations as well as restrictions to the leading dipole-dipole interaction term are no longer sufficient. In this tutorial, we review all relevant aspects of the full calculation of Rydberg interaction potentials. We discuss the derivation of the interaction Hamiltonian from the electrostatic multipole expansion, numerical and analytical methods for calculating the required electric multipole moments and the inclusion of electromagnetic fields with arbitrary direction. We focus specifically on symmetry arguments and selection rules, which greatly reduce the size of the Hamiltonian matrix, enabling the direct diagonalization of the Hamiltonian up to higher multipole orders on a desktop computer. Finally, we present example calculations showing the relevance of the full interaction calculation to current experiments. Our software for calculating Rydberg potentials including all features discussed in this tutorial is available as open source.

By mapping the strong interaction between Rydberg excitations in ultra-cold atomic ensembles onto single photons via electromagnetically induced transparency, it is now possible to realize a medium which exhibits a strong optical nonlinearity at the level of individual photons. We review the theoretical concepts and the experimental state-of-the-art of this exciting new field, and discuss first applications in the field of all-optical quantum information processing.

Random spin-exchange collisions in warm alkali vapor cause rapid decoherence and act to equilibrate the spin state of the atoms in the vapor. In contrast, here we demonstrate experimentally and theoretically a coherent coupling of one alkali species to another species, mediated by these random collisions. We show that the minor species (potassium) inherits the magnetic properties of the dominant species (rubidium), including its lifetime (T1),coherence time (T2), gyromagnetic ratio, and spin-exchange relaxation-free magnetic-field threshold. We further show that this coupling can be completely controlled by varying the strength of the magnetic field. Finally, we explain these phenomena analytically by mode mixing of the two species via spin-exchange collisions.

We suggest a scheme to manipulate paraxial diffraction by utilizing the dependency of a four-wave mixing process on the relative angle between the light fields. A microscopic model for four-wave mixing in a.-type level structure is introduced and compared to recent experimental data. We show that images with feature size as low as 10 mu m can propagate with very little or even negative diffraction. The mechanism is completely different from that conserving the shape of spatial solitons in nonlinear media, as here diffraction is suppressed for arbitrary spatial profiles. At the same time, the gain inherent to the nonlinear process prevents loss and allows for operating at high optical depths. Our scheme does not rely on atomic motion and is thus applicable to both gaseous and solid media.

Standard nonlinear optical materials exhibit negligible nonlinearity at the level of individual photons. We discuss two methods to generate strong photon-photon interactions using either atom-cavity coupling, or strong interactions between atoms in Rydberg states. In particular, we have demonstrated an all-optical transistor gated by one stored photon, and a bound state of two photons.

The fundamental properties of light derive from its constituent particles-massless quanta (photons) that do not interact with one another(1). However, it has long been known that the realization of coherent interactions between individual photons, akin to those associated with conventional massive particles, could enable a wide variety of novel scientific and engineering applications(2,3). Here we demonstrate a quantum nonlinear medium inside which individual photons travel as massive particles with strong mutual attraction, such that the propagation of photon pairs is dominated by a two-photon bound state(4-7). We achieve this through dispersive coupling of light to strongly interacting atoms in highly excited Rydberg states. We measure the dynamical evolution of the two-photon wave-function using time-resolved quantum state tomography, and demonstrate a conditional phase shift(8) exceeding one radian, resulting in polarization-entangled photon pairs. Particular applications of this technique include all-optical switching, deterministic photonic quantum logic and the generation of strongly correlated states of light(9).

The close relation between the processes of paraxial diffraction and coherent diffusion is reflected in the similarity between their shape-preserving solutions, notably the Gaussian modes. Differences between these solutions enter only for high-order modes. Here we experimentally study the behavior of shape-preserving high-order modes of coherent diffusion, known as "elegant" modes, and contrast them with the nonshape-preserving evolution of the corresponding "standard" modes of optical diffraction. Diffusion of the light field is obtained by mapping it onto the atomic coherence field of a diffusing vapor in a storage-of-light setup. The growth of the elegant mode fits well the theoretical expectations.

The realization of strong nonlinear interactions between individual light quanta (photons) is a long-standing goal in optical science and engineering, being of both fundamental and technological significance. In conventional optical materials, the nonlinearity at light powers corresponding to single photons is negligibly weak. Here we demonstrate a medium that is nonlinear at the level of individual quanta, exhibiting strong absorption of photon pairs while remaining transparent to single photons. The quantum nonlinearity is obtained by coherently coupling slowly propagating photons to strongly interacting atomic Rydberg states in a cold, dense atomic gas. Our approach paves the way for quantum-by-quantum control of light fields, including single-photon switching, all-optical deterministic quantum logic and the realization of strongly correlated many-body states of light.

We describe the effect of thermal motion and buffer-gas collisions on a four-level closed N system interacting with strong pump(s) and a weak probe. This is the simplest system that experiences electromagnetically induced absorption (EIA) due to transfer of coherence via spontaneous emission from the excited state to the ground state. We investigate the influence of Doppler broadening, velocity-changing collisions (VCC), and phase-changing collisions (PCC) with a buffer gas on the EIA spectrum of optically active atoms. In addition to exact expressions, we present an approximate solution for the probe absorption spectrum, which provides physical insight into the behavior of the EIA peak due to VCC, PCC, and the wave-vector difference between the pump and probe beams. VCC are shown to produce a wide pedestal at the base of the EIA peak, which is scarcely affected by the pump-probe angular deviation, whereas the sharp central EIA peak becomes weaker and broader due to the residual Doppler-Dicke effect. Using diffusionlike equations for the atomic coherences and populations, we construct a spatial-frequency filter for a spatially structured probe beam and show that Ramsey narrowing of the EIA peak is obtained for beams of finite width.

We derive and measure self-similarly evolving fields under coherent diffusion, analogous to Gaussian modes of optical diffraction. We obtain a quasi-eigenmodes description of polariton dynamics in thermal vapor in the limit of dominating diffusion.

We experimentally demonstrate an optical pumping technique to pump a dilute rubidium vapor into the m_F = 0 ground states. The technique utilizes selection rules that forbid the excitation of the m_F = 0 states by linearly-polarized light. A substantial increase in the transparency contrast of the coherent-population-trapping resonance used for frequency standards is demonstrated.

A new magnetometry method based on electromagnetic induced transparency (EIT) with maximally polarized states is demonstrated. An EIT hyperfine resonance, comprising the m_F = F state (end-state), is observed at a non-zero angle between the laser beam and the magnetic field. The method takes advantage of the process of end-state pumping, a well-known rival of simpler EIT magnetometry schemes, and therefore benefits at a high laser power. An experimental demonstration and a numerical analysis of the magnetometry method are presented. The analysis points on a clear sensitivity advantage of the end-state EIT magnetometer.

Any image, imprinted on a wave field and propagating in free space, undergoes a paraxial diffraction spreading. The reduction or manipulation of diffraction is desirable for many applications, such as imaging, wave-guiding, microlithography and optical data processing. As was recently demonstrated, arbitrary images imprinted on light pulses are dramatically slowed when traversing an atomic medium of electromagnetically induced transparency and undergo diffusion due to the thermal atomic motion. Here we experimentally demonstrate a new technique to eliminate the paraxial diffraction and the diffusion of slow light, regardless of its position and shape. Unlike former suggestions for diffraction manipulation, our scheme is linear and operates in the wavevector space, eliminating the diffraction for arbitrary images throughout their propagation. By tuning the interaction, we further demonstrate acceleration of diffraction, biased diffraction and induced deflection, and reverse diffraction, implementing a negative-diffraction lens. Alongside recent advances in slow-light amplification and image entanglement, diffraction control opens various possibilities for classical and quantum image manipulation.

We study theoretically and experimentally the propagation of slow light in hot atomic vapor and present novel spatial and spectral effects associated with the diffuse atomic motion.

Two-photon processes that involve different sublevels of the ground state of an atom, are highly sensitive to depopulation and decoherence within the ground state. For example, the spectral width of electromagnetically induced transparency resonances in a Λ -type system, are strongly affected by the ground-state depopulation and decoherence rates. We present a direct measurement of decay rates between hyperfine and Zeeman sublevels in the ground state of Rb87 vapor. Similar to the relaxation-in-the-dark technique, pumping lasers are used to prealign the atomic vapor in a well-defined quantum state. The free propagation of the atomic state is monitored using a Ramsey-like method. Coherence times in the range 1-10 ms were measured for room temperature atomic vapor. In the range of the experimental parameters used in this study, the dominant process inducing Zeeman decoherence is the spin-exchange collisions between rubidium atoms.

Reversible and coherent storage of light in an atomic medium is a promising method with possible applications in many fields. In this work, arbitrary two-dimensional images are slowed and stored in warm atomic vapor for up to 30μs, utilizing electromagnetically induced transparency. Both the intensity and the phase patterns of the optical field are maintained. The main limitation on the storage resolution and duration is found to be the diffusion of atoms. A technique analogous to phase-shift lithography is employed to diminish the effect of diffusion on the visibility of the reconstructed image.

We present a theoretical model for electromagnetically induced transparency (EIT) in vapor that incorporates atomic motion and velocity-changing collisions into the dynamics of the density-matrix distribution. Within a unified formalism, we demonstrate various motional effects, known for EIT in vapor: Doppler broadening of the absorption spectrum; Dicke narrowing and time-of-flight broadening of the transmission window for a finite-sized probe; diffusion of atomic coherence during storage of light and diffusion of the light-matter excitation during slow-light propagation; and Ramsey narrowing of the spectrum for a probe and pump beams of finite size.

Dicke narrowing is a phenomenon that dramatically reduces the Doppler width of spectral lines, due to frequent velocity-changing collisions. A similar phenomenon occurs for electromagnetically induced transparency (EIT) resonances, and facilitates ultranarrow spectral features in room-temperature vapor. We directly measure the Dicke-like narrowing by studying EIT line shapes as a function of the angle between the pump and probe beams. The measurements are in good agreement with an analytic theory with no fit parameters. The results show that Dicke narrowing can increase substantially the tolerance of hot-vapor EIT to angular deviations. We demonstrate the importance of this effect for applications such as imaging and spatial solitons using a single-shot imaging experiment, and discuss the implications for the feasibility of storing images in atomic vapor.

We report an experiment in which an optical vortex is stored in a vapor of Rb atoms. Because of its 2π phase twist, this mode, also known as the Laguerre-Gauss mode, is topologically stable and cannot unwind even under conditions of strong diffusion. For comparison, we stored a Gaussian beam with a dark center and a uniform phase. Contrary to the optical vortex, which stays stable for over 100μs, the dark center in the retrieved flat-phased image was filled with light after a storage time as short as 10μs. The experiment proves that higher electromagnetic modes can be converted into atomic coherences and that modes with phase singularities are robust to decoherence effects such as diffusion. This opens the possibility to more elaborate schemes for classical and quantum information storage in atomic vapors.